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eISSN: 2083-5906
ISSN: 1230-1485
ISSN: 1230-1485
ORIGINAL RESEARCH
Determination and Characteristic Analysis
of Atmospheric Carbonyl Compounds
in a North China Plain Hub City
1
School of Municipal and Environmental Engineering, Co-Innovation Center for Green Building of Shandong Province,
Key Laboratory of Renewable Energy Utilization Technologies in Building of Ministry of Education,
Shandong Jianzhu University, Jinan, China
2
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Fudan University, Shanghai, China
3
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, China
4
Jinan Academy of Environmental Sciences, Jinan, China
5
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy
of Environmental Sciences, Beijing, China
Submission date: 2018-08-25
Final revision date: 2018-12-03
Acceptance date: 2018-12-15
Online publication date: 2019-09-10
Publication date: 2019-12-09
Corresponding author
Kai Zhang
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, China
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, China
Pol. J. Environ. Stud. 2020;29(1):861-869
KEYWORDS
TOPICS
ABSTRACT
The concentration and variation trend of atmospheric carbonyl compounds in Jinan were first
measured during autumn 2017 for three continuous weeks at a 3-h time resolution. A total of 14 types
of carbonyls were identified, among which acetone, formaldehyde, and acetaldehyde were the most
abundant carbonyls and their concentrations were 3.75±2.21 ppbv, 2.65±1.67 ppbv, 1.83±1.17 ppbv,
respectively; formaldehyde and acetaldehyde showed similar diurnal variation trends. Butyraldehyde
and isovaleraldehyde were another two important carbonyl compounds with concentrations of
1.05±0.59 ppbv and 1.04±0.47 ppbv, respectively. The average C1/C2 ratio was 1.90, which indicated
that anthropogenic sources were the main contributor of atmospheric carbonyls. The correlation analysis
showed that the measured carbonyls had different sources. Formaldehyde, acetaldehyde, butyraldehyde
and isovaleraldehyde were the most important OVOC contributors to ·OH reactivity and O3 formation.
CONFLICT OF INTEREST
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
CITATIONS (10):
1.
Spatiotemporal patterns and ozone sensitivity of gaseous carbonyls at eleven urban sites in southeastern China
Xin Zhang, Zhenhai Wu, Zhen He, Xuefen Zhong, Fang Bi, Yunfeng Li, Rui Gao, Hong Li, Wenxing Wang
Science of The Total Environment
Xin Zhang, Zhenhai Wu, Zhen He, Xuefen Zhong, Fang Bi, Yunfeng Li, Rui Gao, Hong Li, Wenxing Wang
Science of The Total Environment
2.
Comprehensive observations of carbonyls in the Northern slope of the Tianshan Mountains: Characteristics, reactivity and sources
Kexin Wang, Minghao Dong, Hanran Liu, Xin Zhang, Yunfeng Li, Yafei Wang, Rui Gao, Jingjing Zhang, Yurong Li, Yu Chen, Zhaojiang Li
Air Quality, Atmosphere & Health
Kexin Wang, Minghao Dong, Hanran Liu, Xin Zhang, Yunfeng Li, Yafei Wang, Rui Gao, Jingjing Zhang, Yurong Li, Yu Chen, Zhaojiang Li
Air Quality, Atmosphere & Health
3.
Integrating ambient carbonyl compounds provides insight into the constrained ozone formation chemistry in Zibo city of the North China Plain
Ze Qin, Bo Xu, Zhensen Zheng, Liming Li, Guotao Zhang, Shijie Li, Chunmei Geng, Zhipeng Bai, Wen Yang
Environmental Pollution
Ze Qin, Bo Xu, Zhensen Zheng, Liming Li, Guotao Zhang, Shijie Li, Chunmei Geng, Zhipeng Bai, Wen Yang
Environmental Pollution
4.
Atmospheric chemistry of the coastal area is influenced by the convergence between the inland and marine air: Insight into carbonyl compounds
Jinhe Wang, Ouyang Li, Pengcheng Zhang, Xue Yang, Ravi Yadav, Shan Chen, Yuhong Liu, Chao Zhu, Yangang Ren, Abdelwahid Mellouki
Journal of Environmental Sciences
Jinhe Wang, Ouyang Li, Pengcheng Zhang, Xue Yang, Ravi Yadav, Shan Chen, Yuhong Liu, Chao Zhu, Yangang Ren, Abdelwahid Mellouki
Journal of Environmental Sciences
5.
The pollution levels, variation characteristics, sources and implications of atmospheric carbonyls in a typical rural area of North China Plain during winter
Jinhe Wang, Shuyu Sun, Chongxu Zhang, Chaoyang Xue, Pengfei Liu, Chenglong Zhang, Yujing Mu, Hai Wu, Defa Wang, Hui Chen, Jianmin Chen
Journal of Environmental Sciences
Jinhe Wang, Shuyu Sun, Chongxu Zhang, Chaoyang Xue, Pengfei Liu, Chenglong Zhang, Yujing Mu, Hai Wu, Defa Wang, Hui Chen, Jianmin Chen
Journal of Environmental Sciences
6.
Characteristics and sources of volatile organic compounds during summertime in Tai'an, China
Chengtang Liu, Chenglong Zhang, Junfeng Liu, Pengfei Liu, Yujing Mu
Atmospheric Pollution Research
Chengtang Liu, Chenglong Zhang, Junfeng Liu, Pengfei Liu, Yujing Mu
Atmospheric Pollution Research
7.
Characteristics of atmospheric carbonyls pollution in winter around petrochemical enterprises over North China
Jin-he Wang, Ou-yang Li, Xue Yang, Guang Pan, Guo-lan Fan, Hou-yong Zhang, Zhi-yong Xia, Xiao-yan Sun, Hong-yu Xu, Yan-jun Chen, Chao Zhu
Air Quality, Atmosphere & Health
Jin-he Wang, Ou-yang Li, Xue Yang, Guang Pan, Guo-lan Fan, Hou-yong Zhang, Zhi-yong Xia, Xiao-yan Sun, Hong-yu Xu, Yan-jun Chen, Chao Zhu
Air Quality, Atmosphere & Health
8.
Summertime carbonyl compounds in an urban area in the North China Plain: Identification of sources, key precursors and their contribution to O3 formation
Xue Yang, Gen Zhang, Shuhao Hu, Jinhe Wang, Pengcheng Zhang, Xuelian Zhong, Hengyu Song
Environmental Pollution
Xue Yang, Gen Zhang, Shuhao Hu, Jinhe Wang, Pengcheng Zhang, Xuelian Zhong, Hengyu Song
Environmental Pollution
9.
Molecular Characteristics, Sources, and Health Risk Assessment of Gaseous Carbonyl Compounds in Residential Indoor and Outdoor Environments in a Megacity of Northwest China
Lu Li, Wenting Dai, Minxia Shen, Xinyi Niu, Tafeng Hu, Jing Duan, Junji Cao, Zhenxing Shen, Kin Fai Ho, Jianjun Li, Geun Young Yun
Indoor Air
Lu Li, Wenting Dai, Minxia Shen, Xinyi Niu, Tafeng Hu, Jing Duan, Junji Cao, Zhenxing Shen, Kin Fai Ho, Jianjun Li, Geun Young Yun
Indoor Air
10.
Characteristics, sources and health risk assessment of atmospheric carbonyls during multiple ozone pollution episodes in urban Beijing: Insights into control strategies
Yunfeng Li, Hong Li, Xin Zhang, Yuanyuan Ji, Rui Gao, Zhenhai Wu, Manfei Yin, Lei Nie, Wei Wei, Guohao Li, Yafei Wang, Mei Luo, Hongxiang Bai
Science of The Total Environment
Yunfeng Li, Hong Li, Xin Zhang, Yuanyuan Ji, Rui Gao, Zhenhai Wu, Manfei Yin, Lei Nie, Wei Wei, Guohao Li, Yafei Wang, Mei Luo, Hongxiang Bai
Science of The Total Environment
| eISSN: | 2083-5906 |
| ISSN: | 1230-1485 |
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